杂化钙钛矿中基于表面等离激元的强耦合放大
首发时间:2021-02-05
摘要:该项工作探究了一种存在于由无机-有机钙钛矿纳米线,二氧化硅(SiO2)薄膜,银(Ag)薄膜组成的三明治式的杂化结构中的激子与光子的强耦合作用。表面等离激元的引入使得杂化模式能够减少整个系统的耗散,从而能够增强这种激子与光子的耦合作用。通过计算发现SiO2和Ag薄膜的厚度可以影响耦合强度。当SiO2 (5 nm)和Ag (30 nm)薄膜达到最适宜厚度时,拉比劈裂能量能够达到319 meV,而没有Ag薄膜时拉比劈裂能量仅有270 meV。此外, 在一定范围内,拉比劈裂能量与SiO2薄膜厚度呈线性关系。然而,它与Ag薄膜的厚度呈非线性关系,这是由于杂化模式的有效指数虚部与银薄膜厚度呈非线性关系。该结构为相关实验提供了合适的参数,这些研究结果在设计电泵浦和超低阈值激光器等光学器件方面具有潜在的应用前景。
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Amplification of strong coupling by surface plasmon in a hybridized perovskite
Abstract:This work reports a strong light-matter interaction in a sandwich structure composed of hybridized inorganic-organic perovskite nanowires, silica (SiO2) films, and a silver (Ag) film. Surface plasmon effectively enhances the strong exiton-photon coupling phenomenon, which depends on hybridized modes to reduce the dissipation of the whole system. By caculation it is found that the thickness of SiO2 and Ag films can affect the coupling strength. With the suitable parameters of the SiO2 (5 nm) and Ag (30 nm) films, Rabi splitting can reach 319 meV, while without a Ag film Rabi splitting is only 270 meV. Furthermore, Rabi splitting shows a linear relation with SiO2 film thickness within a limited range. Still, it has a nonlinear relation with Ag film thickness because the imaginary part of the effective index for the hybridized mode shows a nonlinear relation with Ag film thickness. The structure provides suitable parameters for the experiment and has potential application in nano-lasers.
Keywords: Surface Plasmon Perovskite Strong Coupling
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