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期刊论文
The influence of the stretch modes on the classical highly excited bend motion with Darling-Dennison coupling in acetylene
Chemical Physics 269 (2001) 93-99，-0001，（）：
The detail mode characters of the C-H bends with Darling-Dennison coupling in the bath of the stretches of acetylene are analyzed in the coset representative space su(2)/U(1). Besides the local and normal modes, the preces-sionalmode [Mol. Phys. 53 (1984) 961; J Chem Phys. 105 (1996) 10743] is also reproduced. The analysis shows that the excitation of the C-C stretch will lead to more trans local modes for high excitation of the bend This is prone to the isomerization of acetylene to vinylidene
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