黄海平
石油与天然气生成动力学,含油气系统评价及模拟,油气运移和成藏机理及油气藏分布规律,油气成藏后的次生变化及模拟,非烃地球化学,油气田开发地球化学。
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- 姓名:黄海平
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博士生导师
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中医诊断学
- 研究兴趣:石油与天然气生成动力学,含油气系统评价及模拟,油气运移和成藏机理及油气藏分布规律,油气成藏后的次生变化及模拟,非烃地球化学,油气田开发地球化学。
黄海平,男,1962年5月出生,江苏无锡人,留英博士,教授。1985年毕业于江汉石油学院石油地质专业,1988年中国地质大学(北京)硕士研究生毕业,2004年在英国University of Newcastle upon Tyne取得博士学位,导师Steve R Larter教授,论文题目“Effects of biodegradation on crude oil compositions and reservoir profiles in the Liaohe basin, NE China”。1994年破格晋升副教授,1998-1999被国家教委选派到英国University of Aberdeen进修一年,2002年底晋升教授,现正在与加拿大Calgary大学从事联合研究。
主要研究方向:石油与天然气生成动力学,含油气系统评价及模拟,油气运移和成藏机理及油气藏分布规律,油气成藏后的次生变化及模拟,非烃地球化学,油气田开发地球化学。
参加完成了‘八.五’国家重点科技攻关1项,‘973’国家重点攻关1项及横向协作10余项,负责完成国土资源部青年地质行业基金1项,国际合作2项,横向协作近10项。正在负责国家自然科学基金1项;与加拿大Calgary大学国际合作1项;参加加拿大Calgary大学科研1项。
分别获地质矿产部和石油天然气总公司科技成果三等奖各1项,北京市职工技协先进工作者称号1项,中国地质大学教学成果二等奖1项,中国地质大学‘九五’以来优秀科技论文三等奖1项。主要讲授课程:石油与天然气地球化学,储层(油藏)地球化学。
在国际核心期刊第一作者发表SCI论文10余篇,国内核心期刊上发表论文30余篇,其中1999年在《Organic Geochemistry》上发表的一篇论文引用次数已在10次以上,2003年在《Organic Geochemistry》上发表的论文很快被《Nature》引用,在国际同行中产生较大的影响。
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黄海平, Shuichang Zhang a, b, Haiping Huang c, d, *
Organic Geochemistry 36(2005)1204-1214,-0001,():
-1年11月30日
A series of Palaeozoic marine oils ranging from condensates to very heavy oils from the cratonic region of the TarimBasin, NW China have been examined to delineate oil families. Crude oils from the Mesozoic foreland Kuqa Depressionwere also analyzed for comparison. The genetic family was assessed using bulk hydrocarbon isotopic composition,alkylation pattern of polycyclic aromatic hydrocarbons (PAHs) and biomarker distributions. Detailed oil–oil correlationsuggests two distinct families occur in the cratonic region. Despite the diversity of the reservoir rocks and somevariability in oil physical properties, the Tabei and Tazhong oils are classified, in general, into a single family, witha possible indication for secondary subdivision. These oils are characterized by low pristane/phytane (Pr/Ph) ratio, highdibenzothiophene/phenanthrene (DBT/P) ratio, light bulk isotopic composition, high degree of PAH alkylation, highproportion of C23 and C24 tricyclic terpanes and low abundance of C24 tetracyclic terpane and triaromatic dinosteroids.This family is inferred to have a Middle–Upper Ordovician source rock. The Tadong family, distinctly different fromthe Tabei and Tazhong families, is characterized by relatively high Pr/Ph ratio, low DBT/P ratio, slightly heavier bulkisotopic compositions and low degree of PAH alkylation. It also has a unique biomarker signature, with a high proportionof triaromatic dinosteroids, possibly indicating Cambrian–Lower Ordovician source rocks.The oils from the Kuqa Depression are easily distinguished from the other two families due to their terrigenous origin.The major characteristics of the Kuqa oils are high Pr/Ph ratio, very low DBT/P ratio, heavy bulk isotopic composition,low PAH alkylation degree, high proportion of C20 and C21 tricyclic terpanes and C24 tetracylic terpane, andabundance of triaromatic dinosteranes and 4-methyl-24-ethyltriaromatic cholestanes. These characteristics are consistentwith terrestrial organic source rocks deposited under sub-oxic conditions.
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黄海平, Haiping Huang a, b, *, , Bernard F.J. Bowler a, Thomas B.P. Oldenburg a, Steve R. Larter a
Organic Geochemistry 35(2004)1619-1634,-0001,():
-1年11月30日
e biodegradation – ranging from levels 2 to 5 on the [Peters, K.E., Moldowan, J.M., 1993. The BiomarkerGuide: Interpreting Molecular Fossils in Petroleum and Ancient Sediments. Prentice Hall, Englewood Cliffs,NJ, p. 363] scale (abbreviated as _PM level_) -while the shallower Es1 column has undergone more severe biodegradation,ranging from PM level 5 to 8. Both columns show excellent vertical biodegradation gradients, with degree of biodegradationincreasing with increasing depth toward the oil–water contact (OWC). The compositional gradients in theoil columns imply mass transport control on degradation rates, with degradation occurring primarily at the OWC. Thediffusion of hydrocarbons to the OWC zone will be the ultimate control on the maximum degradation rate. The chemicalcomposition and physical properties of the reservoired oils, and the _degradation sequence_ of chemical componentsare determined by mixing of fresh oil with biodegraded oil.The PAH concentrations and molecular distributions in the reservoired oils from these biodegraded columns showsystematic changes with increasing degree of biodegradation. The C3+-alkylbenzenes are the first compounds to bedepleted in the aromatic fraction. Concentrations of the C0-5-alkylnaphthalenes and the C0-3-alkylphenanthrenesdecrease markedly during PM levels 3–5, while significant isomer variations occur at more advanced stages of biodegradation(>PM level 4). The degree of alkylation is a critical factor controlling the rate of biodegradation; in most cases the rate decreaseswith increasing number of alkyl substituents. However, we have observed that C3-naphthalenes concentrations decrease faster than those of C2-naphthalenes, and methylphenanthrenes concentrations decrease faster than that of phenanthrene.Demethylation of a substituted compound is inferred as a possible reaction in the biodegradation process.Differential degradation of specific alkylated isomers was observed in our sample set. The relative susceptibility ofthe individual dimethylnaphthalene, trimethylnaphthalene, tetramethylnaphthalene, pentamethylnaphthalene, methylphenanthrene,dimethylphenanthrene and trimethylphenanthrene isomers to biodegradation was determined. The C20and C21 short side-chained triaromatic steroid hydrocarbons are degraded more readily than their C26-28 long sidechainedcounterparts. The C21-22-monoaromatic steroid hydrocarbons (MAS) appear to be more resistant to biodegradationthan the C27-29-MAS.Interestingly, the most thermally stable PAH isomers are more susceptible to biodegradation than less thermally stableisomers, suggesting that selectivity during biodegradation is not solely controlled by thermodynamic stability and thatsusceptibility to biodegradation may be related to stereochemical structure. Many commonly used aromatic hydrocarbonmaturity parameters are no longer valid after biodegradation toPMlevel 4 although some ratios change later than others.The distribution of PAHs coupled with knowledge of their biodegradation characteristics constitutes a useful probe forthe study of biodegradation processes and can provide insight into the mechanisms of biodegradation of reservoired oil.
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黄海平, Haiping Huanga, b, *, Steve R.Larter a, Bernard F.J. Bowlera, Thomas B.P. Oldenburga
Organic Geochemistry 35(2004)299-316,-0001,():
-1年11月30日
A suite of petroleum reservoir extracts from the Liaohe basin, NE China, was analyzed to investigate the effects andcontrols of biodegradation on petroleum composition.Systematic changes, seen as marked gradients in petroleum bulkcomposition, component concentrations and molecular indicators, have been observed in two biodegraded oil columns.In the Es3 column (1700-1850 m), biodegradation has removed substantial amounts of normal and isoprenoid alkanes.More severe biodegradation occurs in the shallower Es1 column (1500-1650m), with both steranes and hopanes beingpartially removed.Temperature has an overall control on biodegradation in the two columns, a lower reservoir temperatureleading to a higher degree of biodegradation.However, observed variation in the degree of biodegradation inthe Es3 column at different sites is controlled by water leg size, with a higher level of degradation being associated witha thicker water leg.The supply of nutrients from the water leg is thought to have a significant impact upon the degreeof biodegradation.In addition to water leg size/nutrient supply, the compositional gradients also are controlled by therelative rate of mixing of fresh oil charge.Gradients can only be conserved in biodegraded petroleum columns ifthe rate of diffusive mixing is similar to or lower than the rate at which the hydrocarbons are removed.A biodegradationmodel is proposed that couples geochemical and geological factors to provide a coherent approach forassessing the impact of degradation on petroleum.Our geochemical study indicates that biodegradation occurs mainlywithin a narrow region at or near the base of the oil column.The stable compositional gradients are produced after aninitial induction period involving diffusive transport of alkanes to the oil-water contact (OWC) and diffusion of biodegradationproducts such as 25-norhopanes and other metabolites away from the reaction site.The mixing of continuously-charged oil with 'residential' biodegraded oil by diffusion may be considered as one of the most importantfactors controlling the biodegradation process.The conceptual model illustrates all of these processes and opens thepossibility of model-driven prediction of oil properties and 'sweetspot' location in reservoirs.
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【期刊论文】Geochemistry of natural gases in deep strata of theSongliao Basin, NE China
黄海平, Haiping Huanga, b, *, Jie Yanga, c, Yufeng Yangd, Xiujuan Dua, d
International Journal of Coal Geology 58(2004)231-244,-0001,():
-1年11月30日
Chemical composition and stable carbon isotopic studies were undertaken for 27 gas samples from deep strata of theXujiaweizi Depression in the Songliao Basin to investigate their origin. Gas molecular and carbon isotopic compositions showgreat variety. Methane is the main component for all studied samples and its content ranges from 57.4% to 98.2% with anaverage of 90.1%. Gas wetness ranges from 0.8% to 16.7% with an average of 2.7%. The main non-hydrocarbon gases arecarbon dioxide and nitrogen with an average of 4.0% and 3.2%, respectively. Carbon isotope data suggest that these deep stratagases are mainly coal-type gases mixed with minor amounts of associated (oil-type) gases. Coal-type gases are characterized byheavier carbon isotopic values and drier chemical compositions. These gases were generated from the Lower CretaceousShahezi Formation coals interbedded shales with type III kerogen during the postmature stage of hydrocarbon generation. Oiltypegases are characterized by lighter carbon isotope and higher wetness, which were generated from the Lower Cretaceousshales with type II kerogen in the shallow strata during the early mature stage of hydrocarbon generation. Mixing of twodifferent gases causes unusual carbon isotopic distribution patterns, with lighter isotopic values in higher numbered carbons inmost gases. The discovery of coal-type gases in the Songliao Basin provides new prospects for the exploration in this region.
Coal-type gas, Carbon isotopic composition, Maturity, Mixing, Songliao Basin
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黄海平, Haiping Huanga, b, Steve R. Lartera, Gordon D. Lovea, *
Organic Geochemistry 34(2003)1673-1687,-0001,():
-1年11月30日
A detailed organic geochemical study; utilising petrography, biomarker hydrocarbon analysis and high temperatureGC analysis of extractable wax hydrocarbon constituents was performed on four marginally oil window-mature sourcerocks from the Shahejie Formation (Eocene), Damintun depression in eastern China. The main maceral components inthe source rocks were vitrinite, liptinite and exinite, with vitrinite being more abundant (>50 vol.%) in organic-leansamples whose TOC contents were between 1 and 2 wt.%. Large differences in pristane/phytane ratios suggested thatthe organic-rich samples were deposited in a less oxic depositional environment than that for the organic-lean rocks.The distribution of extractable wax hydrocarbons, determined by high temperature GC, showed a marked differencebetween these two sample types. The organic-rich samples contained high molecular weight hydrocarbons (HMWHCs)dominated by macrocrystalline n-alkanes (n-C23–n-C37, typically maximising at n-C29), while the organic-lean samplescontained lower amounts of extractable wax hydrocarbons but were relatively rich in microcrystalline components (>n-C35). In all source rocks (Es3 and Es4), a noticeable odd-over-even predominance (OEP) of n-alkane chain lengths(up to n-C65) was evident, consistent with a direct biological origin for the long n-alkyl chains. They were mostprobably formed during diagenesis from decarboxylation of predominantly even-carbon-numbered aliphatic acidsoriginating from higher plant or lacustrine algal sources and/or were directly biosynthesised in hydrocarbon form. Atleast two other homologous series of branched/cyclic HMWHCs were observed, one of which was confirmed as a seriesof branched alkanes (probably methyl-branched). The carbon number distribution patterns of HMWHCs may be primarilycontrolled by thermal maturity and biogenic source input as well as being influenced by diagenetic reactionsgoverned by depositional environmental conditions, as shown previously [Carlson, R.M.K., Teerman, S.C., Moldowan,J.M., Jacobson, S.R., Chan, E.I., Dorrough, K.S., Seetoo, W.C., Mertani, B., 1993. High temperature gas chromatographyof high wax oils. In: Indonesian Petroleum Association, 22nd Annual Convention Proceedings. Jakarta, Indonesian,pp. 483–507. Carlson, R.M.K., Jacobsen, S.R., Moldowan, J.M., Chan E.I., 1994. Potential application of hightemperature gas chromatography to Middle Eastern petroleum exploration and production. In: Al-Husseini, M.I.(Ed.), Geo'94, Vol 1., Selected Middle East Papers from The Middle East Petroleum Geoscience Conference, 1994; Gulf PetroLink. Manama, Bahrain, pp. 258–267]. Our study indicates for the first time that Es3 source rocks as well asEs4 facies contain HMWHCs. The distributions of extractable wax hydrocarbons suggest that both Es4 and Es3members may potentially serve as important parent source rocks for generating waxy petroleum in this region.
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【期刊论文】Origin of an unusual heavy oil from the Baiyinchagan depression,Erlian basin, northern China
黄海平, Haiping Huanga, b, *, Guangxi Jina, c, Changsong Lina, Yabin Zhenga
Marine and Petroleum Geology 20(2003)1-12,-0001,():
-1年11月30日
A detailed organic geochemical analysis of six oil samples from the Baiyinchagan depression in the Erlian basin, Northern China, wascarried out in order to evaluate their origin. The oils are reservoired at a very shallow depth (223-560 m subsurface) and their chemical andphysical properties vary greatly, ranging from normal to extremely heavy oil. The preservation of non-biodegraded oil in such a shallowreservoir is possibly related with palaeo-pasteurization of the reservoir before uplift. Maturity difference is not the primary control on thechemical and physical properties of the oils and there is considerable geochemical evidence to suggest the additional influence of inreservoir/post-accumulation processes such as biodegradation, water-washing and (possibly) evaporation. Whereas some oils appear to beless affected, others are moderately biodegraded up to level 4 on the Peters and Moldowan (1993) scale, with sterane distributions largelyunaffected and 25-norhopanes undetected. Contrary to classical biodegradation, the unusual heavy oil shows little evidence of biodegradationfrom aliphatic components. Water-washing is suggested to be the primary process leading to its formation since the severe alteration ofsoluble aromatic hydrocarbons is observed. In addition, since the oils have been uplifted significantly after accumulation, evaporation and/orleakage to modify oil compositions cannot be ruled out.
Biodegradation, Water-washing, Heavy oil, Erlian basin
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黄海平, Haiping Huanga, b, Bernard F.J. Bowlera, Zhanwen Zhangc, Thomas B.P. Oldenburga, Steve R. Lartera, *
Organic Geochemistry 34(2003)951-969,-0001,():
-1年11月30日
rease slightly during theearly stages of biodegradation and then sharply decrease after level 4, when preferential depletion of alkylated carbazolescompared to benzocarbazoles and dibenzocarbazoles or naphthocarbazoles is observed. The susceptibility of alkylated carbazoleisomers to biodegradation decreases with increasing carbon number of the alkyl substituents. Furthermore, nitrogen(N–H) shielded or partially shielded compounds substituted in the 1 and/or 8 positions seem more susceptible to biodegradationthan their nitrogen-exposed counterparts. For example, biodegradation resulted in the preferential removal of 1-methylcarbazole relative to the other methylcarbazole isomers and among the dimethylcarbazoles; 1,8-dimethylcarbazoleseems more susceptible to biodegradation than other isomers, even though some exceptions do occur in our sample set.The benzocarbazole ratio [Nature 383 (1996) 593] decreased with increasing degree of biodegradation. Benzo[b]carbazolehas the highest apparent ability to resist biodegradation among the benzocarbazole isomers.
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【期刊论文】Influence of biodegradationon benzocarbazole distributionsin reservoired oils
黄海平, HUANG Haiping, , REN Fangxiang, & S.R. Larter
Chinese Science Bulletin Vol. 47 No.20 October 2002,-0001,():
-1年11月30日
Partition coefficient difference of benzocarbazoleisomers between oil, water and mineral phase makesthem a useful indicator to quantify petroleum migrationdistance. Because of their nitrogen-heteroatom andannelated aromatic cycles they are generally regarded asbeing more resistant and the effects of biodegradation ontheir concentrations and distributions have not previouslybeen investigated. Reservoir extracts from three wells locatedin the Leng 43 block of the Liaohe Basin were analyzedto investigate their occurrence and the effect of biodegradation.Both hydrocarbon biomarkers and benzocarbazoleisomers show systematical changes with the increase extentof biodegradation in study columns. Carbazole compoundsmay be biodegraded in a similar way to that observed inaliphatic and aromatic hydrocarbons. The distance from oilwater contact is a primary control factor for biodegradation.The concentrations of benzocarbazole isomers show a slightincrease in the upper part of the columns then a sharp decreasetowards oil water contact (OWC). Among three isomersbenzo[a]carbazole seems more susceptible to biodegradationthan other two isomers and benzo[b]carbazole hashigher ability to resist bacterial attack. Benzo[b]carbazole/benzo- [a]carbazole ratios can sensitively indicate thedegree of biodegradation and the benzocarbazole index (BCratio) cannot be directly used as a migration indicator inbiodegraded oils.
carbazoles, benzocarbazoles, biodegradation, LiaoheBasin.,
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【期刊论文】松辽盆地徐家围子断陷深层天然气同位素倒转现象研究
黄海平
地球科学——中国地质大学学报,2000,25(6):617~623,-0001,():
-1年11月30日
天然气的同位素组成受源岩有机质类型、热演化程度和成藏后的次生变化等多种因素的影响,其单体烃同位素分布特征是区分各种因素影响程度的地球化学指纹。天然气单体烃同位素通常有随碳数增加而变重的趋势,而徐家围子深层天然气单体烃同位素倒转现象却比较普遍,高地温和细菌氧化对于造成该区同位素倒转的可能性不大,浅层油型气或无机气的混合作用没有充分的地质证据,同层有机质中不同类型气的混合和盖层微渗漏造成的蒸发分馏作用可能是导致徐家围子断陷深层天然气同位素倒转的主要原因。
天然气成因, 同位素倒转, 混合作用, 微渗漏, 蒸发分馏作用, 徐家围子断陷.,
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黄海平, Haiping Huang, Michael J. Pearson*
Organic Geochemistry 30(1999)1455-1470,-0001,():
-1年11月30日
The applicability of sulphur aromatic parameters, based on ratios of dibenzothiophene (DBT) and its alkylatedhomologues, as indicators of oil maturity has been investigated in 27 oils from the Damintun and Zhuanhua Depres-sions, Bohai Bay Basin. The oils were characterised by bulk composition and environmentally-sensitive aliphatic bio-markers and were derived from a wide range of lacustrine source depositional environments ranging from highlyreducing hypersaline (sulphur-rich oils) to terrestrial input-dominated freshwater (very high wax oils) with maturitiesranging from immature to probable mid-mature. Dibenzothiophene-based maturity parameters are not well-correlatedwith sterane isomerization ratios, and immature oils, in particular, could not be discriminated by these aromaticmaturity indicators. In contrast, DBT-based parameters are strongly-correlated with pristane to phytane and Ts/Tmratios. High methyldibenzothiophene ratios (MDR) are associated with fresh water source deposition whilst lowMDRs are found in oils of hypersaline source affnity. Unusually high relative concentrations of 2+3-MDBT wereobserved in some of the immature oils inferred to be sourced by lacustrine organic laminites. The data provide furtherevidence that thermal stress is not the sole factor controlling the distribution patterns of dibenzothiophenes in oils andthat source depositional environments can exert a dominant in
Dibenzothiophene, Palaeoenvironment, Lacustrine, Hypersaline, High wax, Immature oil
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