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2011年06月09日

【期刊论文】Biomass pyrolysis/gasification for product gas production: the overall investigation of parametric effects

陈冠益, G. Chen a, *, J. Andries a, Z. Luo b, H. Spliethoff a

Energy Conversion and Management 44 (2003) 1875-1884,-0001,():

-1年11月30日

摘要

The conventional biomass pyrolysis/gasification process for production of medium heating value gas for industrial or civil applications faces two disadvantages, i.e. low gas productivity and the accompanying corrosion of downstream equipment caused by the high content of tar vapour contained in the gas phase. The objective of this paper is to overcome these disadvantages, and therefore, the effects of the operating parameters on biomass pyrolysis are investigated in a laboratory setup based on the principle of keeping the heating value of the gas almost unchanged. The studied parameters include reaction temperature, residence time of volatile phase in the reactor, physico-chemical pretreatment of biomass particles, heating rate of the external heating furnace and improvement of the heat and mass transfer ability of the pyrolysis reactor. The running temperature of a separate cracking reactor and the geometrical configuration of the pyrolysis reactor are also studied. However, due to time limits, different types of catalysts are not used in this work to determine their positive influences on biomass pyrolysis behaviour. The results indicate that product gas production from biomass pyrolysis is sensitive to the operating parameters mentioned above, and the product gas heating value is high, up to 13–15 MJ/Nm3.

Biomass, Pyrolysis/, gasification, Parameters, Effect, Product gas

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2011年06月09日

【期刊论文】Biomass gasification integrated with pyrolysis in a circulating fluidised bed

陈冠益, G. Chen a, b, *, J. Andries b, H. Spliethoff b, M. Fang c, P.J. van de Enden b

Solar Energy 76 (2004) 345-349,-0001,():

-1年11月30日

摘要

The use of biomass for energy generation is getting increasing attention. At present, gasification of biomass is taken as a popular technical route to produce fuel gas for application in boilers, engine, gas turbine or fuel cell. Up to now, most of researchers have focused their attentions only on fixed-bed gasification and fluidised bed gasification under airblown conditions. In that case, the producer gas is contaminated by high tar contents and particles which could lead to the corrosion and wear of blades of turbine. Furthermore, both the technologies, particularly fixed bed gasification, are not flexible for using multiple biomass-fuel types and also not feasible economically and environmentally for large scale application up to 10-50 MWth. An innovative circulating fluidised bed concept has been considered in our laboratory for biomass gasification thereby overcoming these challenges. The concept combines and integrates partial oxidation, fast pyrolysis (with an instantaneous drying), gasification, and tar cracking, as well as a shift reaction, with the purpose of producing a high quality of gas, in terms of low tar level and particulates carried out in the producer gas, and overall emissions reduction associated with the combustion of producer gas. This paper describes our innovative concept and presents some experimental results. The results indicate that the gas yield can be above 1.83 Nm3/kg and the fluctuation of the gas yield during the period of operation is 3.3% at temperature of 750℃ Generally speaking, the results achieved support our concept as a promising alternative to gasify biomass for the generation of electricity.

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