Atomistic molecular dynamics simulations were performed to investigate the dependence of the self-diffusivity of liquid carbon tetrachloride (CCl4) confined in pillared pore materials on the pore width, porosityand the surface heterogeneityof the solid walls. The simulated results show that the self-diffusivityof liquid CCl4 does not increase monotonicallywith the pore width, but in an cillatorymanner to approach the bulk diffusivity. Moreover, the presence of activated sites characterizing the surface heterogeneity and the pillars reduces the self-diffusivityof liquid CCl4 confined in pillared pores. The effects of these factors on the self-diffusivityof fluids should be taken into account when a porous nanomaterial is designed or chosen for a certain process, in addition to their effects on other properties such as the adsorption capability.