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【期刊论文】Catalyst preparation using plasma technologies
刘昌俊, Chang-jun Liu a, *, Gheorghi P. Vissokov b, Ben W.-L. Jang c
Catalysis Today 72(2002)173-184,-0001,():
-1年11月30日
This paper discusses catalyst preparation using thermal and cold plasmas. In general, there are three main trends in preparing catalysts using plasma technologies: (1) plasma chemical synthesis of ultrafine particle catalysts; (2) plasma assisted deposition of catalytically active compounds on various carriers, especially plasma spraying for the preparation of supported catalysts; (3) plasma enhanced preparation or plasma modification of catalysts. Compared to conventional catalyst preparation, there are several advantages of using plasmas, including: (1) a highly distributed active species; (2) reduced energy requirements; (3) enhanced catalyst activation, selectivity, and lifetime; (4) shortened preparation time. These advantages are leading to many potential applications of plasma prepared catalysts.
Plasma preparation, Catalyst, Plasma modification, Plasma spraying, Thermal plasma, Cold plasma
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刘昌俊, Chang-jun Liu a, b, *, Kailu Yu a, Yue-ping Zhang b, Xinli Zhu a, Fei He a, Baldur Eliasson b, c
Catalysis Communications 4(2003)303-307,-0001,():
-1年11月30日
A novel Pd/HZSM-5 catalyst was prepared first by glow discharge plasma treatment followed by calcination thermally. Such prepared catalyst shows a higher activity and an enhanced stability for methane combustion. The XRD characterization and XPS analysis confirm that the plasma preparation leads to a better preparation of PdO active species over the HZSM-5 support. Especially, a plasma-enhanced acidity has been achieved upon the FT-IR analysis. The enhanced acidity plays an important role in stabilizing the dispersed PdO active species on the zeolite support.
Pd/, HZSM-5, Plasma treatment, Glow discharge, Methane, Combustion
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【期刊论文】Modification of starch by glow discharge plasma
刘昌俊, Ji-Jun Zou a, Chang-Jun Liu a, *, Baldur Eliasson b
Carbohydrate Polymers 55(2004)23-26,-0001,():
-1年11月30日
A novel method for starch modification is investigated. Starch is highly cross linked by glow discharge plasma, without the assistance of conventional chemical agents, thus avoiding any environmental concerns. An energy-charge-transfer mechanism is suggested for the function of plasma. This process could be useful for the production of large quantities of modified starch.
Starch, Modification, Crosslinking, Glow discharge, Plasma
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刘昌俊, Tao Jiang a, Chang-Jun Liu a, ), Ming-Fa Rao b, Chun-De Yao b, Guo-Liang Fan c
Fuel Processing Technology 73Ž2001.143-152,-0001,():
-1年11月30日
A diesel fuel additive has been synthesized from conversion of dimethyl ether(DME) using dielectric barrier dischargeŽDBD.plasma at atmospheric pressure and low temperatures. A high conversion of DME has been achieved. The product of such conversion is a mixture of hydrocarbons and oxygenates that can be used as high-performance diesel fuel additives. The maximum conversion of DME reached 47.2% with a selectivity of liquid product (a mixture of dimethoxy-containing hydrocarbons) more than 39.0% at 1208C and a 30 mlrmin flow rate of DME.
Dielectric-barrier discharges, Diesel fuel additives, Dimethyl ether, Dimethoxy propane, Dimethoxy ethane
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【期刊论文】Non-thermal plasma approaches in CO utilization
刘昌俊, Chang-jun Liu a, *, Gen-hui Xu a, Timing Wang b
Fuel Processing Technology 58(1999)119-134,-0001,():
-1年11月30日
CO2 is the final product of combustion of all fossil fuels. CO2 itself has little value by far, but it contributes more than 50% to the man-made greenhouse effect among all the greenhouse gases. There is still no proven technology for the chemical utilization of such a plentiful carbon resource. Recently, non-thermal plasmas have been found to be effective in the activation of CO2 for the formation of more valuable hydrocarbons. The non-thermal plasma approaches can even be performed at ambient condition. In this review, the present state of carbon dioxide utilization via non-thermal plasmas is addressed.
Non-thermal plasma, CO2, Greenhouse effect
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