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【期刊论文】Nonlinear Saturable Absorption of Liquid‐Exfoliated Molybdenum/Tungsten Ditelluride Nanosheets
Small,2016,12(11):1489-1497
2016年01月22日
Molybdenum disulfide (MoS2) and tungsten disulfide (WS2), two representative transition metal dichalcogenide materials, have captured tremendous interest for their unique electronic, optical, and chemical properties. Compared with MoS2 and WS2, molybdenum ditelluride (MoTe2) and tungsten ditelluride (WTe2) possess similar lattice structures while having smaller bandgaps (less than 1 eV), which is particularly interesting for applications in the near‐infrared wavelength regime. Here, few‐layer MoTe2/WTe2 nanosheets are fabricated by a liquid exfoliation method using sodium deoxycholate bile salt as surfactant, and the nonlinear optical properties of the nanosheets are investigated. The results demonstrate that MoTe2/WTe2 nanosheets exhibit nonlinear saturable absorption property at 1.55 μm. Soliton mode‐locking operations are realized separately in erbium‐doped fiber lasers utilizing two types of MoTe2/WTe2‐based saturable absorbers, one of which is prepared by depositing the nanosheets on side polished fibers, while the other is fabricated by mixing the nanosheets with polyvinyl alcohol and then evaporating them on substrates. Numerous applications may benefit from the nonlinear saturable absorption features of MoTe2/WTe2 nanosheets, such as visible/near‐infrared pulsed laser, materials processing, optical sensors, and modulators.
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Advanced Materials,2015,27(44):7162-7167
2015年10月08日
All‐inorganic colloidal cesium lead halide perovskite quantum dots (CsPbX3, X = Cl, Br, I) are revealed to be a new class of favorable optical‐gain materials, which show combined merits of both colloidal quantum dots and halide perovskites. Low‐threshold and ultrastable stimulated emission is demonstrated under atmospheric conditions with wavelength tunability across the whole visible spectrum via either size or composition control.
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【期刊论文】Quantum Dot Light‐Emitting Diodes Based on Inorganic Perovskite Cesium Lead Halides (CsPbX3)
Advanced Materials,2015,27(44):7162-7167
2015年10月07日
Novel quantum‐dot light‐emitting diodes based on all‐inorganic perovskite CsPbX3 (X = Cl, Br, I) nanocrystals are reported. The well‐dispersed, single‐crystal quantum dots (QDs) exhibit high quantum yields, and tunable light emission wavelength. The demonstration of these novel perovskite QDs opens a new avenue toward designing optoelectronic devices, such as displays, photodetectors, solar cells, and lasers.
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NPG Asia Materials,2015,7():e168
2015年03月27日
Three-dimensional (3D) nanostructures assembled with one- or few-layered ultrathin two-dimensional (2D) crystals have triggered great interest in energy and environmental applications. Here, we introduce a gas-foaming process in an hexagonal boron nitride (h-BN) ceramic material to fabricate 3D white graphene (WG) foams without using any catalysts or templates for superstrong pollutant removal applications. Importantly, the introduction of vesicants guaranteed the reproducibility and yield (>500 cm3). Interestingly, these 3D WG foams possessed a vesicular structure with hierarchical pores ranging from nm to μm scales and with ultrathin walls consisting of mono- or few-layered BN membranes with planar sizes as large as 100 μm. Consequently, such microstructure merits of hierarchical pores and ultrathin walls endowed them not only very low density (2.1 mg cm−3) but also superstrong adsorption ability, illustrated by capacitances up to 190 times its own weight toward a wide range of environment contaminations, including various oils and dyes. Thus, the 3D h-BN WG foams prepared by vesicant-assisted foaming should have great potential as outstanding environmental scavengers.
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Angew. Chem. In. Ed. ,2014,54(6):1759-1764
2014年09月11日
As an important energy‐saving technique, white‐light‐emitting diodes (W‐LEDs) have been seeking for low‐cost and environment‐friendly substitutes for rare‐earth‐based expensive phosphors or Pd2+/Cd2+‐based toxic quantum dots (QDs). In this work, precursors and chemical processes were elaborately designed to synthesize intercrossed carbon nanorings (IC‐CNRs) with relatively pure hydroxy surface states for the first time, which enable them to overcome the aggregation‐induced quenching (AIQ) effect, and to emit stable yellow‐orange luminescence in both colloidal and solid states. As a direct benefit of such scarce solid luminescence from carbon nanomaterials, W‐LEDs with color coordinate at (0.28, 0.27), which is close to pure white light (0.33, 0.33), were achieved through using these low‐temperature‐synthesized and toxic ion‐free IC‐CNRs as solid phosphors on blue LED chips. This work demonstrates that the design of surface states plays a crucial role in exploring new functions of fluorescent carbon nanomaterials.
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