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2004年12月28日

【期刊论文】用激光增益获取弱增益拉曼模式的受激拉曼散射光谱*

普小云, 杨正, 江楠, 陈永康, 戴宏

物理学报,2003,52(10):2443-06,-0001,():

-1年11月30日

摘要

当酒精的弱增益拉曼模式处于罗丹明640染料分子的激光增益范围时,在由悬垂液滴构成的圆形谐振腔中,观察到乙醇分子C—H伸缩系列模中多个弱增益拉曼模式的受激拉曼散射(SRS)光谱。随着抽运光的增强,迅速增长的强增益拉曼模式的受激辐射抑制了其他弱增益模式的SRS,并导致染料激光的完全淬灭。通过分析圆形腔腔模的光子速率方程和激光染料分子的三能级粒子数速率方程,解释了观察到的实验现象。

受激拉曼散射,, 悬垂液滴,, 弱拉曼增益模式,, 激光增益

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2004年12月28日

【期刊论文】ArF Laser Induced Plasma Spectroscopy of Lead Ions in Aqueous Solutions: Plume Reheating with a Second Nd: YAG Laser Pulse

普小云, X. Y. PU* and N. H. CHEUNG†

,-0001,():

-1年11月30日

摘要

Laser-induced breakdown spectroscopy, ArF laser ablation, Plasma reheating, Lead, Aqueous samples.,

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2004年12月28日

【期刊论文】Sensitive elemental analysis of aqueous colloids by laser-induced plasma spectroscopy

普小云, X. Y. Pu, a) W. Y. Ma, b) and N. H. Cheung c)

,-0001,():

-1年11月30日

摘要

Highly sensitive elemental analysis of lead carbonate colloids was demonstrated by two-pulse laser-induced plasma spectroscopy. The first laser pulse created a vapor plume with the particulates concentrated in space because of their slower propagation. They were then ablated by an ArF laser pulse that efficiently atomized and excited the lead analyte. The lead emissions were much enhanced, while the background continuum interference was minimized. The detection limit for lead was shown to be 14.2 ppb, compared with 13 ppm achieved by conventional laser-induced breakdown spectroscopy of lead ions in water and 210 ppb for lead aerosols.

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2004年12月28日

【期刊论文】LASING FROM A DYE-DOPED PENDANT DROP AND ITS PRECESSION

普小云, Pu XIAO-YUN (普小云) a)b) and LEE WING-KEE (李荣基) b)

,-0001,():

-1年11月30日

摘要

We have observed lasing from the rim of dye-doped ethylene glycol pendant drops. Sptatial-resolved spectral measurements show that the lasing wavelength varies along a vertical rim of the drop. Time-resolved measurements indicate that lasing precession occurs within the drop. Various lasing patterns due to lasing precession are explained. The measured precession periods for different pumping points are in good agreement with the calculated values based on morphology-dependent resonance theory.

pendant drop,, lasing precession,, red shift

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2004年12月28日

【期刊论文】Enhancement of stimulated Raman scattering of weak-gain Raman modes in a pendant drop by dye-lasing gain

普小云, Xiao-Yun Pu and Zheng Yang, Wing-Kee Lee

,-0001,():

-1年11月30日

摘要

The enhancement of stimulated Raman scattering (SRS) of weak-gain Raman modes in pendant drops is accomplished by overlapping Stokes wavelengths of the Raman modes with the Rhodamine 640 dye-lasing gain region (called the gain-overlap method). The dye concentration and the pumping intensity of frequencydoubled Nd: YAG lasers determine the efficiency of the enhancement. We apply the gain-overlap technique at optimal dye concentration and pump intensity to probe minority species in pendant drops formed by binary mixtures. The limits of detectable concentrations of the minority species, methanol in methanol-ethanol and ethanol in ethanol-water (dye-doped) mixtures, are much less than those in undoped mixtures. The smooth fluorescence-lasing spectral curves emitted from dye-doped pendant drops reduce complications in distinguishing SRS signals from quasi-periodic fluorescence-lasing spectra in microdroplets.

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    云南大学,云南

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